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Re: PEM fuel cell efficiency

Subject: Re: PEM fuel cell efficiency
From: "G. R. L. Cowan"
Date: Sat, 30 Jul 2005 15:02:46 -0400
Newsgroups: sci.energy.hydrogen
"Don W." included:
> 
> 
> ... If I understand correctly, the HHV of hydrogen is ALL the potential
> chemical energy contained in the hydrogen, including the fraction that is
> unrecoverable except as low grade heat because the "oxidized hydrogen" is
> formed as a gas and not as a liquid.  The LHV of hydrogen is the five
> sixths of the energy that is not necessarily "exothermic" (MIGHT be
> recovered in some form other than heat.)  Is this understanding correct?
> 
> IF that is correct, then it seems proper (to me, anyway) to use HHV and say
> that the maximum possible efficiency of the fuel cell is 83% instead of
> using the LHV and saying that the maximum possible efficiency of the fuel
> cell is 100% even though there is heat in excess of that 100% dissipated in
> or slightly after the fuel cell.
> 
> Others disagree.  Here is a link with some good information that says
> Ballard is right to use HHV in calculating the efficiency of their fuel
> cells:
> http://planetforlife.com/h2/h2fuelcell.html

I tend to use the delta 'G', -228.3 kJ/mol 
for hydrogen oxidation yielding water vapour, 
-237.15 kJ/mol for hydrogen oxidation yielding liquid water. 
This small difference reflects the fact that water 
at 25 C isn't very far from its boiling point, 
where the difference would be zero.

If there were a perfectly efficient electrolyser 
it would put in exactly 228.3 kJ of DC electricity 
to get a mole of hydrogen out of a mole of water vapour ... 
or 237.15 kJ to get one out of liquid water. 

A little low-grade heat would be absorbed here and re-released here; 
looking only at DG, one doesn't see this and doesn't have to 
deal with ideal efficiencies of 83 percent or 120 percent.

Instead, ideal machine efficiency is simply 100 percent. 
A perfectly efficient fuel cell would get all of that 237 kJ 
or all of the 228 kJ back. 

The only real air-breathing ones for which I know of published 
data that can be made to yield an efficiency get 93.5 kJ/mol. 

But having the oxygen come pure from a tank makes a big difference, 
so that the submarine claims might be enthusiastic 
by only five percentage points, or ten. 15, tops. For sure, tops. 
Fairly sure.

When air-breathing, you have to pump the air; 
oxygen from a LOX tank pumps itself, 
and if you don't count the cold vapour's expansion potential 
as part of the onboard energy, you get the sort of 
efficiency number a brochure writer likes. 

I have no precise efficiency measurement for any specific 
pure-oxygen fuel cell, so I suppose they too are about 
10 points below the range that is commonly quoted,
low 60s to 70 percent, without, of course, 
saying percent of what.

I did once look at how much a 60-percent-of-DG cell, 
if one existed, would lose if it had to purify its own 
oxygen. Hydrogen takes 252.0 g oxygen per kilowatt-hour 
of -DG. By the above hypothesis a cell can make 600 Wh 
with this. Oxygen from zeolite PSA oxygen purifiers 
costs 0.645 Wh/g, so the 252.0 g costs 162.5 Wh, 
dropping us to 440 Wh, 44 percent. 

The same 16-percentage-point deduction would apply 
to whatever real efficiency real pure-oxygen fuel cells have.


--- Graham Cowan, former hydrogen fan
                                www.eagle.ca/~gcowan/Paper_for_11th_CHC.html">http://www.eagle.ca/~gcowan/Paper_for_11th_CHC.html --
boron as energy carrier: real-car range, nuclear cachet

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